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Preparation of Multicolour Solid Fluorescent Carbon Dots for Light-Emitting Diodes Using Phenylethylamine as a Co-Carbonization Agent

文献类型： 外文期刊

作者： An, Yulong 1 ; Liu, Can 1 ; Li, Yan 1 ; Chen, Menglin 1 ; Zheng, Yunwu 1 ; Tian, Hao 3 ; Shi, Rui 2 ; He, Xiahong 2 ; Lin, Xu 1 ;

作者机构： 1.Southwest Forestry Univ, Natl Joint Engn Res Ctr Highly Efficient Utilizat, Kunming 650224, Yunnan, Peoples R China

2.Southwest Forestry Univ, Key Lab Forest Resources Conservat & Utilizat Sou, Minist Educ, Kunming 650224, Yunnan, Peoples R China

3.Yunnan Acad Agr Sci, Agroprod Proc Res Inst, Kunming 650000, Yunnan, Peoples R China

关键词： carbon dots; solid fluorescence; solvent control; multicolour; optoelectronic applications

期刊名称：INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES （ 影响因子：6.208； 五年影响因子：6.628 ）

ISSN：

年卷期： 2022 年 23 卷 19 期

页码：

收录情况： SCI

摘要： Carbon dots (CDs), as a new type of photoluminescent nanomaterial, have attracted extensive attention in various fields because of their unique luminescence properties. However, CDs will exhibit fluorescence quenching in the solid state or aggregate state, which limits their application. In this paper, a unique strategy is proposed to regulate solutions to achieve multicolour fluorescence of CDs in the solid state. We report the successful preparation of orange, green and blue solid fluorescent CDs using citric acid, urea and phenylethylamine as precursors and methanol, ethanol and water as solvents, respectively. The solid-state fluorescence of CDs may be caused by the linkage of the phenylethyl structure to the surface of CDs during formation, which effectively disperses the CDs and prevents pi-pi interactions between graphitized nuclei. Meanwhile, multicolour solid fluorescent CDs are realized by adjusting the solvent in the preparation process. Based on the excellent fluorescence properties of CDs, orange, green and blue light-emitting diodes (LEDs) are prepared. A white LED (WLED) can be obtained by mixing the three colours of solid fluorescent CDs, which shows the application potential of CDs in display lighting equipment.

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